This paper investigates the supervisory control of nondeterministic discrete event systems to enforce bisimilarity with respect to deterministic specifications. A notion of synchronous simulation-based controllability is introduced as a necessary and sufficient condition for the existence of a bisimilarity enforcing supervisor, and a polynomial algorithm is developed to verify such a condition. When the existence condition holds, a supervisor achieving bisimulation equivalence is constructed. Furthermore, when the existence condition does not hold, two different methods are provided for synthesizing maximal permissive sub-specifications.